Experimental study of the effect of dissolution on the gas diffusion layer in polymer electrolyte membrane fuel cells

Taehun Ha, Junhyun Cho, Jaeman Park, Kyoungdoug Min, Han Sang Kim, Eunsook Lee, Jy Young Jyoung

Research output: Contribution to journalArticlepeer-review

42 Scopus citations

Abstract

The gas diffusion layer (GDL) is important for maintaining the performance of polymer electrolyte membrane (PEM) fuel cells, as its main function is to provide the cells with a path for fuel and water. In this study, the mechanical degradation process of the GDL was investigated using a leaching test to observe the effect of water dissolution. The amount of GDL degradation was measured using various methods, such as static contact angle measurements and scanning electron microscopy. After 2000 h of testing, the GDL showed structural damage and a loss of hydrophobicity. The carbon-paper-type GDL showed weaker characteristics than the carbon-felt-type GDL after dissolution because of the structural differences, and the fuel cell performance of the leached GDL showed a greater voltage drop than that of the fresh GDL. Contrary to what is generally believed, the hydrophobicity loss of GDL was not caused by the decomposition of polytetrafluoroethylene (PTFE).

Original languageEnglish
Pages (from-to)12427-12435
Number of pages9
JournalInternational Journal of Hydrogen Energy
Volume36
Issue number19
DOIs
StatePublished - Sep 2011

Keywords

  • Degradation
  • Durability
  • Gas diffusion layer
  • Polymer electrolyte membrane fuel cell

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